ADOPTED LEVELS, GAMMAS for 254No

Author: Balraj Singh |  Citation: Nucl. Data Sheets 156, 1 (2019) |  Cutoff date: 31-Jan-2019 

 Full ENSDF file | Adopted Levels (PDF version) 


Q(β-)=-5150 keV SYS(n)= 7707 keV 12S(p)= 3740 keV SYQ(α)= 8226 keV 8
Reference: 2017WA10

References:
  A  254Lr ε decay (18.1 S)  B  258Rf α decay (12.0 MS)
  C  254No IT decay (265 MS)  D  254No IT decay (184 μs):GSI
  E  254No IT decay (184 μs):LBNL  F  208Pb(48Ca,2nγ):PROMPT γ

General Comments:

Production and assignment of 254No isotope:

1958Gh40, 1966Do04: parent of 250Fm; chemistry

1966Do04: 238U(22Ne,6n); excitation function

1966Za04: 243Am(15N,4n); parent of 250Fm

1967Gh01: 246Cm(12C,4n); excitation function

1967Mi03: 242Pu(16O,4n); excitation function

1988Tu07: 208Pb(48Ca,2n); chemistry; grandparent of 246Cf

Consult the NSR database at www.nndc.bnl.gov for numerous papers since 1988 for the production cross sections of 254No in different reactions

2018It04: measured mass excess=84675 keV 42(stat) 19(syst) using multireflection time-of-flight mass spectrograph at GARIS-RIKEN facility. This value can be compared to evaluated mass excess of 84723.4 keV 93 in 2017Wa10

2012Mi27: measured mass excess using time-of-flight ion-cyclotron-resonance method

2010Bl04, 2010Bl03, 2010Dw01: measured mass using SHIPTRAP Penning trap spectrometer at GSI

Theoretical studies: consult the NSR database at www.nndc.bnl.gov for 100 references dealing with theoretical calculations of half-lives for different decay modes, binding energies, fission characteristics, level properties, moments and deformations.

Levels: The decay scheme of the 184-μs isomer has been studied by 2010He10 at GSI, and by 2010Cl01 at LBNL. Very different decay schemes were proposed in the two experiments, although a similar rotational band, but with different Jπ values and configuration, was assigned in both the studies. 2016WaZW conducted an independent experiment at Jyvaskyla (JYFL) to resolve the difference between the two studies. The author favored the decay scheme given by 2010He10, with a possible difference that the 605-keV transition deexcited the isomer directly rather than through an intermediate level as suggested by 2010He10. However, 2016WaZW concluded with the following statement about the 605-keV transition: "The 605 keV rays seen at the focal plane in coincidence with the decay of the fast isomer confirm that there is a transition with this energy in 254No somewhere between the two isomers, but it does not give any more information about where in the level scheme the transition should be placed. Any of the level schemes in figure 9.1 is consistent with this observation ". Evaluator also consulted Prof. R.-D. Herzberg, thesis advisor of 2016WaZW, as well as the first author of 2006He19 paper for his opinion on the current status of the decay scheme of this isomer. Evaluator was advised (ref. e-mail reply of June 19, 2017 from Prof. Herzberg) that at this time, no definite decay scheme could be adopted, and that future experiments with more advanced detector arrays are needed to investigate the decay scheme between the two isomers: 184 μs and 265 ms. Thus, while the two currently proposed decay schemes are presented in this evaluation as separate datasets, no decay scheme has been adopted in this dataset.

Q-value: Estimated uncertainties (2017Wa10): 300 for Q(β-), 30 for S(p)

Q-value: S(2n)=14291 13, S(2p)=6670 11 (2017Wa10)










E(level)
(keV)
XREFJπ(level) T1/2(level)E(γ)
(keV)
I(γ)M(γ)Final Levels
     0.0 BC    0+ 51.2 s 4 
% ε = 10 1
% α = 90 1
% SF = 0.17 2
     
    44.2 4  BCDEF 2+      44.2 4 S
  100
[E2]
     0.0
0+
   145.2 7   CDEF 4+     101.1 6 
  100
E2
    44.2
2+
   304.6 7   CDEF 6+     159.5 2 
  100
E2
   145.2
4+
   518.7 7   CDEF 8+     214.1 1 
  100
E2
   304.6
6+
   786.0 8      F 10+     267.3 1 
  100
E2
   518.7
8+
   987.5 8   CDEF (3+)     842 1 
  943 1 
   36 9 
  100 16 


   145.2
    44.2
4+
2+
  1033.2 11   CDE  (4+)      45S
  887
 
 


   987.5
   145.2
(3+)
4+
  1091.1 9   CDE  (5+)      58S
  103
  786 1 
 
 
 



  1033.2
   987.5
   304.6
(4+)
(3+)
6+
  1104.1 8      F 12+     318.1 2 
  100
(E2)
   786.0
10+
  1160.3 9   CDE  (6+)      69
  126
  856
 
 
 



  1091.1
  1033.2
   304.6
(5+)
(4+)
6+
  1243.1 9   CDE  (7+)      82
  151
  940
  100
  110 40 
 



  1160.3
  1091.1
   304.6
(6+)
(5+)
6+
  1296.4 11   CDE  (8-) 265 ms 2 
% IT = 100
% SF = 0.020 12
% α ≤ 0.01
   53
  778
  100 7 
   14 4 
(E1)
[E1]
  1243.1
   518.7
(7+)
8+
  1407.8 11    DE  (9-)     111.4 2 
  100
[M1]
  1296.4
(8-)
  1470.7 8      F 14+     366.6 2 
  100
[E2]
  1104.1
12+
  1530.8 15    DE  (10-)     123
 

  1407.8
(9-)
E(level)
(keV)
XREFJπ(level) T1/2(level)E(γ)
(keV)
I(γ)M(γ)Final Levels
  1530.8+X   DE  J1        
  1664.4+X 1    DE  J1+1     133.3 1 
  100

  1530.8+X
J1
  1809.1+X 8    DE  J1+2     145 1 
  100

  1664.4+X
J1+1
  1883.4 8      F 16+     412.7 2 
  100
[E2]
  1470.7
14+
  1966.1+X 8    DE  J1+3     156.9 2 
  302
  100 17 
 


  1809.1+X
  1664.4+X
J1+2
J1+1
  2134.4+X 8    DE  J1+4     168.5 1 
  325.5 5 
  100 17 
   83 33 


  1966.1+X
  1809.1+X
J1+3
J1+2
  2314.8+X 8    DE  J1+5     179.5 1 
  347.2 2 
  100 13 
   76 22 


  2134.4+X
  1966.1+X
J1+4
J1+3
  2314.8+Y   DE  (16) 184 µs 3 
% IT = 100
% SF ≤ 0.012
     
  2339.4 9      F 18+     456.0 3 
 

  1883.4
16+
  2837.4 14      F (20+)     498 1 
 

  2339.4
18+
  3373.4 17      F (22+)     536 1 
 

  2837.4
(20+)
  3943.4 20 ?     F (24+)     570?
 

  3373.4
(22+)

E(level): From least-squares fit to Eγ data, assuming uncertainty of 1 keV when not stated.

Jπ(level): From band structures as proposed in several studies using 208Pb(48Ca,2nγ) reaction. Members of the ground-state from 4+ to 12+ are supported by E2 intraband transitions, higher members from continuing γ cascade.

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Band Transitions:

E(level)
(keV)
Jπ(level) T1/2(level)E(γ)I(γ)M(γ)Final Levels
Band 1 - Kπ=0+, g.s. band.
     0.0 0+ 51.2 s 4 
% ε = 10 1
% α = 90 1
% SF = 0.17 2
     
    44.2 4  2+      44.2 4 S
  100
[E2]
     0.0
0+
   145.2 7  4+     101.1 6 
  100
E2
    44.2
2+
   304.6 7  6+     159.5 2 
  100
E2
   145.2
4+
   518.7 7  8+     214.1 1 
  100
E2
   304.6
6+
   786.0 8  10+     267.3 1 
  100
E2
   518.7
8+
  1104.1 8  12+     318.1 2 
  100
(E2)
   786.0
10+
  1470.7 8  14+     366.6 2 
  100
[E2]
  1104.1
12+
  1883.4 8  16+     412.7 2 
  100
[E2]
  1470.7
14+
  2339.4 9  18+     456.0 3 
 

  1883.4
16+
  2837.4 14  (20+)     498 1 
 

  2339.4
18+
  3373.4 17  (22+)     536 1 
 

  2837.4
(20+)
  3943.4 20  (24+)     570?
 

  3373.4
(22+)
E(level)
(keV)
Jπ(level) T1/2(level)E(γ)I(γ)M(γ)Final Levels
Band 2 - π1/2[521]~#π7/2[514],Kπ=(3+) band
   987.5 8  (3+)        
  1033.2 11  (4+)      45S
  887
 
 


   987.5
   145.2
(3+)
4+
  1091.1 9  (5+)      58S
  103
  786 1 
 
 
 



  1033.2
   987.5
   304.6
(4+)
(3+)
6+
  1160.3 9  (6+)      69
  126
  856
 
 
 



  1091.1
  1033.2
   304.6
(5+)
(4+)
6+
  1243.1 9  (7+)      82
  151
  940
  100
  110 40 
 



  1160.3
  1091.1
   304.6
(6+)
(5+)
6+
E(level)
(keV)
Jπ(level) T1/2(level)E(γ)I(γ)M(γ)Final Levels
Band 3 - Kπ=(8-) band
  1296.4 11  (8-) 265 ms 2 
% IT = 100
% SF = 0.020 12
% α ≤ 0.01
     
  1407.8 11  (9-)     111.4 2 
  100
[M1]
  1296.4
(8-)
  1530.8 15  (10-)     123
 

  1407.8
(9-)
E(level)
(keV)
Jπ(level) T1/2(level)E(γ)I(γ)M(γ)Final Levels
Band 4 - ΔJ=1 band
  1530.8+X J1        
  1664.4+X 1  J1+1     133.3 1 
  100

  1530.8+X
J1
  1809.1+X 8  J1+2     145 1 
  100

  1664.4+X
J1+1
  1966.1+X 8  J1+3     156.9 2 
  302
  100 17 
 


  1809.1+X
  1664.4+X
J1+2
J1+1
  2134.4+X 8  J1+4     168.5 1 
  325.5 5 
  100 17 
   83 33 


  1966.1+X
  1809.1+X
J1+3
J1+2
  2314.8+X 8  J1+5     179.5 1 
  347.2 2 
  100 13 
   76 22 


  2134.4+X
  1966.1+X
J1+4
J1+3

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Additional Gamma Data:













E(level)
(keV)
Jπ(level)T1/2(level)E(γ)
(keV)
MultipolarityConversion
Coefficient
Additional Data
    44.2 2+      44.2 4 [E2]1510α=1510 70
   145.2 4+     101.1 6 E230.0α=30.0 10
   304.6 6+     159.5 2 E23.94α=3.94
   518.7 8+     214.1 1 E21.204α=1.204
   786.0 10+     267.3 1 E20.535α=0.535
  1104.1 12+     318.1 2 (E2)0.300α=0.300
  1296.4 (8-) 265 ms 2 
% IT = 100
% SF = 0.020 12
% α ≤ 0.01
   53(E1)0.83α=0.83 5
(8-) 265 ms 2 
% IT = 100
% SF = 0.020 12
% α ≤ 0.01
  778[E1]0.0085α=0.0085
  1407.8 (9-)     111.4 2 [M1]9.51α=9.51
  1470.7 14+     366.6 2 [E2]0.195α=0.195
  1883.4 16+     412.7 2 [E2]0.1397α=0.1397

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Additional Level Data and Comments:

E(level)Jπ(level)T1/2(level)Comments
     0.00+ 51.2 s 4 
% ε = 10 1
% α = 90 1
% SF = 0.17 2
Measured %ε=10 1, %SF=0.23 10 (2010He10) from the number of α decays and fission events from 254No and the number of α decays from 254Fm.
E(level): Measured %ε=10 1, %SF=0.23 10 (2010He10) from the number of α decays and fission events from 254No and the number of α decays from 254Fm. Kπ=0+, g.s. band.
    44.22+   E(level): Kπ=0+, g.s. band.
   145.24+   E(level): Kπ=0+, g.s. band.
   304.66+   E(level): Kπ=0+, g.s. band.
   518.78+   E(level): Kπ=0+, g.s. band.
   786.010+   E(level): Kπ=0+, g.s. band.
   987.5(3+)   E(level): π1/2[521]~#π7/2[514],Kπ=(3+) band.
  1033.2(4+)   E(level): π1/2[521]~#π7/2[514],Kπ=(3+) band.
  1091.1(5+)   E(level): π1/2[521]~#π7/2[514],Kπ=(3+) band.
  1104.112+   E(level): Kπ=0+, g.s. band.
  1160.3(6+)   E(level): π1/2[521]~#π7/2[514],Kπ=(3+) band.
  1243.1(7+)   E(level): π1/2[521]~#π7/2[514],Kπ=(3+) band.
  1296.4(8-) 265 ms 2 
% IT = 100
% SF = 0.020 12
% α ≤ 0.01
unobservedGammaIntensity=49 2:From 254No IT decay (265 ms).
E(level): unobservedGammaIntensity=49 2:From 254No IT decay (265 ms). Kπ=(8-) band.
  1407.8(9-)   E(level): Kπ=(8-) band.
  1470.714+   E(level): Kπ=0+, g.s. band.
  1530.8(10-)   E(level): Kπ=(8-) band.
  1530.8+XJ1   J1=10- in 2010He10, 10+ in 2010Cl01.
E(level): ΔJ=1 band.
  1664.4+XJ1+1   E(level): ΔJ=1 band.
  1809.1+XJ1+2   E(level): ΔJ=1 band.
  1883.416+   E(level): Kπ=0+, g.s. band.
  1966.1+XJ1+3   E(level): ΔJ=1 band.
  2134.4+XJ1+4   E(level): ΔJ=1 band.
  2314.8+XJ1+5   E(level): ΔJ=1 band.
  2314.8+Y(16) 184 µs 3 
% IT = 100
% SF ≤ 0.012
See 2015Ko14 evaluation for γ-transition hindrance factors, where the isomer is considered to deexcite directly through the 605γ.
  2339.418+   E(level): Kπ=0+, g.s. band.
E(level)Jπ(level)T1/2(level)Comments
  2837.4(20+)   E(level): Kπ=0+, g.s. band.
  3373.4(22+)   E(level): Kπ=0+, g.s. band.
  3943.4(24+)   E(level): Kπ=0+, g.s. band.

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Additional Gamma Comments:

E(level)E(gamma)Comments
   987.5   842I(γ): Relative branching ratios of 842γ and 943γ are from 254No IT decay (265 ms)
   943I(γ): Relative branching ratios of 842γ and 943γ are from 254No IT decay (265 ms)
  1243.1    82I(γ): Relative branching ratios of 842γ and 943γ are from 254No IT decay (265 ms)
   151I(γ): Relative branching ratios of 842γ and 943γ are from 254No IT decay (265 ms)
  1296.4    53I(γ): Relative branching ratios of 842γ and 943γ are from 254No IT decay (265 ms)
   778I(γ): Relative branching ratios of 842γ and 943γ are from 254No IT decay (265 ms)
  1407.8   111.4E(γ): average of 111.4 2 in 254No IT decay (184 μs):GSI, and 111.4 3 in 254No IT decay (184 μs):LBNL
  1664.4+X   133.3E(γ): average of 133.3 1 in 254No IT decay (184 μs):GSI, and 133.4 4 in 254No IT decay (184 μs):LBNL
  1809.1+X   145E(γ): from 254No IT decay (184 μs):LBNL
  1966.1+X   156.9E(γ): average of 156.9 2 in 254No IT decay (184 μs):GSI, and 156.9 3 in 254No IT decay (184 μs):LBNL
   302E(γ): from 254No IT decay (184 μs):GSI
  2134.4+X   168.5E(γ): average of 168.5 1 in 254No IT decay (184 μs):GSI, and 168.9 3 in 254No IT decay (184 μs):LBNL
I(γ): Branching ratios from 254No IT decay (184 μs):LBNL
   325.5E(γ): 325 in 254No IT decay (184 μs):GSI, and 325.5 5 in 254No IT decay (184 μs):LBNL
I(γ): Branching ratios from 254No IT decay (184 μs):LBNL
  2314.8+X   179.5E(γ): average of 179.5 1 in 254No IT decay (184 μs):GSI, and 179.4 3 in 254No IT decay (184 μs):LBNL
   347.2E(γ): average of 347.1 2 in 254No IT decay (184 μs):GSI, and 347.5 5 in 254No IT decay (184 μs):LBNL
I(γ): average of 57 22 in 254No IT decay (184 μs):GSI, and 100 {25 in 254No IT decay (184 μs):LBNL

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