ADOPTED LEVELS for 222U
Authors: Balraj Singh, M.S. Basunia, Jun Chen Et Al., | Citation: Nucl. Data Sheets 192, 315 (2023) | Cutoff date: 25-Sep-2023
Full ENSDF file | Adopted Levels (PDF version)
Q(β-)=-7000 keV 60 | S(n)= 8320 keV 90 | S(p)= 3390 keV 80 | Q(α)= 9480 keV 50 | ||
Reference: 2021WA16 |
E(level) (keV) | Jπ(level) | T1/2(level) |
0 | 0+ | 4.6 µs 7 % α ≈ 100 |
Additional Level Data and Comments:
E(level) | Jπ(level) | T1/2(level) | Comments |
0 | 0+ | 4.6 µs 7 % α ≈ 100 | Measured Eα=9.31 MeV 5 from the decay of 222U to 218Th (2015Kh09), 9246 keV 8 (2023Lu04). Evaluator’s note: the difference in the two values seems significant, however, it seems that the uncertainty of 8 keV in 2023Lu04 is underestimated, as this value was deduced from simply a spread of Eα values (without uncertainties) for only five events (#3, #4, #5, #6 and #9) in authors’ Table I. E(level): Measured Eα=9.31 MeV 5 from the decay of 222U to 218Th (2015Kh09), 9246 keV 8 (2023Lu04). Evaluator’s note: the difference in the two values seems significant, however, it seems that the uncertainty of 8 keV in 2023Lu04 is underestimated, as this value was deduced from simply a spread of Eα values (without uncertainties) for only five events (#3, #4, #5, #6 and #9) in authors’ Table I. |
1983Hi12: W(40Ar,xn) E(40Ar)=180 MeV; products were separated from the primary beam by the velocity filter; parent of 214Ra (7.16-MeV α). Tentative identification of 222U nuclide.
2012Ya04: 100Mo(124Sn,2n)222U,E(124Sn)=505 MeV. Measured evaporation residues at the HRIBF-ORNL facility. Deduced production σ=21 nb +38-21 from in-beam data, and <270 nb from post-irradiation collection of decay product 206Po (from α decay chain: 222U |) 218Th |) 214Ra |) 210Rn |) 206Po). No confirmed production and identification of 222U nuclide.
2015Kh09: 222U produced and identified in 176Yb(50Ti,4n), E(50Ti)=231-255 MeV reaction. The 50Ti12+ pulsed beam was produced by the UNILAC at GSI. Target=0.45 mg/cm2 5 thick 176YbF3 mounted on a rotating wheel, synchronized with the beam pulses. Evaporation residues (ERs), separated by using gas-filled TransActinide Separator and Chemistry Apparatus (TASCA) with flight time of 0.53 μs 6 through the separator, were implanted in a double-sided silicon strip detector. The events due to radioactive decays of implanted residues were selected from the events related to beam using a multiwire proportional counter (MWPC). Measured Eα, Iα, from Er-α correlated events from subsequent α-decay chains, half-lives of the parent nuclei corresponding to the evaporation residues, and successive α-decay daughters, the latter identified by their known characteristics in literature. The identification of 222U was made based on observed Er-α, two- or three-signal correlated events using a fast data acquisition and combined analog and digital (CANDI) readout system. α total of 81 Er traces were recorded for 222U and analyzed with subsequent α decay chain: 222U -> 218Th -> 214Ra. FWHM≈40 keV for 8.7 MeV α particles, recorded as single events, ≈110 keV and ≈180 keV for multiple α events stored in a single trace with time differences of 1 μs and 0.17 μs, respectively. Deduced α-decay reduced widths, and neutron shell gap, the latter compared with FRDM95 and HFB26 theoretical calculations for the Z=82-92,n=126 nuclei
2023Lu04: 222U produced in 186W(40Ar,4n),E(40Ar)=188 MeV, followed by the separation of the evaporation residues (ERs) using the He-filled recoil separator SHANS at the HRIFL-Lanzhou facility. Measured α-α-correlated decay chains, Eα and T1/2 for the decay of the g.s. of 222U from a total of ten observed events. Deduced reduced α-decay width and hindrance factor in Rasmussen’s formalism.
Nuclear structure calculations:
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2021Gu26: calculated odd-even mass differences using deformed mean-field plus extended pairing model.
2021No02, 2021Ro02: calculated low-energy levels, Jπ, B(E1), B(E2), B(E3), quadrupole and octupole deformation parameters using Hartree-Fock-Bogoliubov approximation, based on the Gogny-D1M energy density functional and corresponding mapped sdf-IBM.
2020Ca18: calculated deformation parameters β2, β3, octupole deformation energies, proton moments Q20 and Q30 using five Skyrme energy density functionals, and four covariant energy density functionals
2017Xi15: calculated levels, Jπ, B(E1), B(E2), B(E3), electric dipole moments, deformation energy surface in (β3,β3) plane using microscopic quadrupole-octupole collective Hamiltonian (QOCH) based on relativistic α(p)-PK1 energy density functional and δ-interaction pairing.
2016Ag06: calculated equilibrium β2, β3 deformation parameters for ground state using density functional models and ε2, ε3 parameters by mic-mac (MM) approach, potential energy surfaces in (β2,β3) plane using CEDF DD-PC1 theory, and covariant energy density functionals, with a nonlinear meson coupling, with density-dependent meson couplings, and pairing correlations within relativistic Hartree-Bogoliubov theory.
Theoretical calculations for α and cluster decays:
2022He18: calculated α-decay T1/2, α-preformation factor using density-dependent cluster model with RMF NN interactions, M3Y NN interactions and universal decay law (UDL) formula.
2022Xu13: calculated α-decay T1/2 using the Gamow model with a screened electrostatic barrier.
2021Sa52: calculated Q(2α), T1/2 for 2α-decay with and without the deformation effects using used modified generalized liquid drop model, and Coulomb and proximity potential model with different preformation factors for double α decay.
2021Se10: calculated Q(β-)values and T1/2 for cluster decays, change in neutron-skin thickness, the isospin-asymmetry using self-consistent Hartree-Fock-Bogolyubov based on Skyrme-SLy4 effective nucleon-nucleon interaction
2020Ni01, 2017Ni01: calculated α-branching ratios to vibrational states, α-decay T1/2, partial half-lives for β+/ε and α-decay modes using multichannel cluster model (MCCM).
2018Se01: calculated driving potential vs cluster charge, T1/2 for α-decay and for cluster decay, α and cluster Q values using Skyrme-SLy4 nucleon-nucleon interaction, within the frame work of the performed cluster model
2017Sa39: calculated cluster decay T1/2 using 12 different potentials
Q-value: Q(ε)=2210 100, Q(εp)=40 50, S(2n)=14880 110 (syst), S(2p)=4990 50 (2021Wa16)