Skip to main content
Log in

Quantification of radioisotopes produced in 1.4 GeV proton irradiated lead–bismuth eutectic targets

  • Regular Article – Experimental Physics
  • Published:
The European Physical Journal A Aims and scope Submit manuscript

Abstract

Six cylindrical lead bismuth eutectic (LBE) targets having fixed diameter of 6 mm and varying lengths of 8–50 mm were irradiated with a 1.4 GeV proton beam at CERN-ISOLDE. Both short-lived (\(5\hbox { h } {<}\hbox {T}_{1/2} {<}5\hbox { days}\)) and long-lived (\(\hbox {T}_{1/2} {>}5\hbox { days}\)) radionuclides were identified by off-line \(\upgamma \)-spectrometry and their activities at the end of bombardment (EOB) were determined. Total 80 \(\upgamma \)-emitting radionuclides, ranging from \(^{7}\hbox {Be}\) to \(^{209}\hbox {At}\), were identified in the 50 mm long LBE target. The yields of all the radioisotopes were compared with the Monte Carlo Code FLUKA. The spallation reaction was the dominant mode whereas fission induced reactions had no significant contribution. The high energy proton irradiated LBE target may act as a large source of several clinically important and other exotic radionuclides.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7

Similar content being viewed by others

Data Availability Statement

This manuscript has no associated data or the data will not be deposited. [Authors’ comment: All data produced in the experiment have been used in this manuscript.]

References

  1. H. Klein, Proc. Int. Linac Conf., Japan, 322–327 (1994)

  2. J. Buongiorno, C. Larson, K.R. Czerwinski, Radiochim. Acta 91, 153 (2003)

    Article  Google Scholar 

  3. D. Choudhury, S. Lahiri, Appl. Radiat. Isot. 137, 33 (2018)

    Article  Google Scholar 

  4. S. Lahiri, M. Maiti, ISOLDE workshop and Users Meeting, November 18-20, CERN, Geneva, Switzerland (2009)

  5. Y. Tall, S. Cormon, M. Foucher, A. Guertin, T. Kirchner, L. Zanini, M. Andersson, K. Berg, H. Franberg, F. Groschel, E. Manfrin, W. Wagner, M. Wohlmuther, P. Everaerts, U. Koster, H. Ravn, E.N. Messomo, C. Jost, Y. Kojima, Int. Conf. Nucl. Data Sci. Technol. (2007). https://doi.org/10.1051/ndata:07762

    Article  Google Scholar 

  6. B. Hammer, J. Neuhausen, V. Boutellier, M. Wohlmuther, A. Türler, D. Schumann, Anal. Chem. 87, 5656 (2015)

    Article  Google Scholar 

  7. J. Neuhausen, U. Köster, B. Eichle, Radiochim. Acta 92, 917 (2004)

    Article  Google Scholar 

  8. M. Rizzi, J. Neuhausen, R. Eichler, A. Türler, T. Mendonça, T. Stora, B. Gonzalez Prieto, A. Aerts, D. Schumann, J. Nucl. Mater. 450, 304 (2014)

    Article  Google Scholar 

  9. M. Maiti, K. Ghosh, T.M. Mendonca, T. Stora, S. Lahiri, J. Radioanal. Nucl. Chem. 302, 1003 (2014)

    Article  Google Scholar 

  10. A. Ferrari, P.R. Sala, A. Fasso, J. Ranft, CERN-2005-10, INFN/TC\(\_\)05/11, SLAC-R-773 (2005)

  11. T.T. Böhlen, F. Cerutti, M.P.W. Chin, A. Fasso, A. Ferrari, P.G. Ortega, A. Mairani, P.R. Sala, G. Smirnov, V. Vlachoudis, Nucl. Data Sheets 120, 211 (2014)

    Article  ADS  Google Scholar 

  12. L.M. Oranj, T. Kakavand, M. Sadeghi, M.A. Rovias, Nucl. Instrum. Methods Phys. Res. A 677, 22 (2012)

    Article  ADS  Google Scholar 

  13. G. Battistoni, F. Broggi, M. Brugger, M. Campanella, M. Carboni, A. Empl, A. Fasso, E. Gadioli, F. Cerutti, A. Ferrari, M. Lantz, A. Mairani, M. Margiotta, C. Morone, S. Muraro, K. Parodi, V. Patera, M. Pelliccioni, L. Pinsky, J. Ranft, S. Roesler, S. Rollet, P.R. Sala, M. Santana, L. Sarchiapone, M. Sioli, G. Smirnov, F. Sommerer, C. Theis, S. Trovati, R. Villari, H. Vincke, V. Vlachoudis, J. Volaire, N. Zapp, Nucl. Instrum. Methods Phys. Res. B 269, 2850 (2011)

    Article  ADS  Google Scholar 

  14. G. Battistoni, J. Bauer, T.T. Boehlen, F. Cerutti, M.P.W. Chin, R.D.S. Augusto, A. Ferrari, P.G. Ortega, W. Kozlowska, G. Magro, A. Mairani, K. Parodi, P.R. Sala, P. Schoofs, T. Tessonnier, V. Vlachoudis, Front Oncol. 6, 1 (2016)

    Article  Google Scholar 

  15. F. Botta, A. Mairani, G. Battistoni, M. Cremonesi, A.D. Dia, A. Fasso, A. Ferrari, M. Ferrari, G. Paganelli, G. Pedroli, M. Valente, Med. Phys. 38, 3944 (2011)

    Article  Google Scholar 

  16. D. Choudhury, S. Lahiri, Eur. Phys. J. A 54, 212 (2018)

    Article  ADS  Google Scholar 

  17. R. Augusto, L. Buehler, Z. Lawson, S. Marzari, M. Stachura, T. Stora, Appl. Sci. 4, 265 (2014)

    Article  Google Scholar 

  18. https://www.physik.uzh.ch/~matthias/espace-assistant/manuals/en/anleitung-ab_e.pdf

  19. L. Zanini, Summary Report for MEGAPIE R&D Task Group X9: Neutronic and Nuclear Assessment, PSI (2005)

  20. L. Fiorito, A. Stankovskiy, A. Hernandez-Solis, G.V. Eynde, G. Zerovnik, EPJ Nucl. Sci. Technol. 4, 48 (2018)

    Article  ADS  Google Scholar 

  21. C. Müller, K. Zhernosekov, U. Köster, K. Johnston, H. Dorrer, A. Hohn, N. Walt, A. Türler, R. Schibli, J. Nucl. Med. 53, 1951 (2012)

    Article  Google Scholar 

  22. M. Maiti, S. Lahiri, B.S. Tomar, Radiochim. Acta 99, 527 (2011)

    Article  Google Scholar 

  23. A.N. Moiseeva, R.A. Aliev, V.N. Unezhev, V.A. Zagryadskiy, S.T. Latushkin, N.V. Aksenov, N.S. Gustova, M.G. Voronuk, GYa. Starodub, A.A. Ogloblin, Sci. Rep. 10, 508 (2020)

    Article  ADS  Google Scholar 

  24. M. Maiti, S. Lahiri, J. Radioanal. Nucl. Chem. 283, 637 (2010)

    Article  Google Scholar 

  25. C. Brihaye, M. Guillaume, N. Lavi, M. Cogneau, J. Nucl. Med. 23, 1114 (1982)

    Google Scholar 

  26. K. Ghosh, M. Maiti, S. Lahiri, Radiochim. Acta 105, 747 (2017)

    Article  Google Scholar 

  27. K. Ghosh, S. Lahiri, M. Maiti, J. Radioanal. Nucl. Chem. 310, 1345 (2016)

    Article  Google Scholar 

  28. B. Dutta, S. Lahiri, B.S. Tomar, Sep. Sci. Technol. 48, 2468 (2013)

    Article  Google Scholar 

  29. D. Choudhury, N. Naskar, S. Lahiri, Radiochim. Acta 106, 743 (2018)

    Article  Google Scholar 

  30. D. Nayak, S. Lahiri, A. Ramaswami, Appl. Radiat. Isot. 57, 483 (2002)

    Article  Google Scholar 

  31. Y. Nagame, H. Nakahara, Y. Murakami, Int. J. Appl. Radiat. Isot. 30, 669 (1979)

    Article  Google Scholar 

  32. M. Maiti, S. Lahiri, Z. Szűcs, J. Radioanal. Nucl. Chem. 307, 1667 (2016)

    Article  Google Scholar 

  33. L. Gastaldo, K. Blaum, K. Chrysalidis, T.D. Goodacre, A. Domula, M. Door, H. Dorrer, ChE Duellmann, K. Eberhardt, S. Eliseev, C. Enss, A. Faessler, P. Filianin, A. Fleischmann, D. Fonnesu, L. Gamer, R. Haas, C. Hassel, D. Hengstler, J. Jochum, K. Johnston, U. Kebschull, S. Kempf, T. Kieck, U. Koester, S. Lahiri, M. Maiti, F. Mantegazzini, B. Marsh, P. Neroutsos, Yu N. Novikov, P.C.O. Ranitzsch, S. Rothe, A. Rischka, A. Saenz, O. Sander, F. Schneider, S. Scholl, R.X. Schuessler, Ch. Schweiger, F. Simkovic, T. Stora, Z. Szucs, A. Tuerler, M. Veinhard, M. Weber, M. Wegner, K. Wendt, K. Zuber, Eur. Phys. J. Spec. Top. 226, 1623 (2017)

    Article  Google Scholar 

  34. D. Choudhury, S. Lahiri, N. Naskar, J. Radioanal. Nucl. Chem. 314, 2551 (2017)

    Article  Google Scholar 

  35. D. Choudhury, S. Lahiri, J. Radioanal. Nucl. Chem. 318, 1967 (2018)

    Article  Google Scholar 

  36. D. Choudhury, S. Lahiri, T. Nag, S. Sodaye, A. Bombard, J. Radioanal. Nucl. Chem. 324, 897 (2020)

    Article  Google Scholar 

Download references

Acknowledgements

We acknowledge fruitful discussions with Professor Sukalyan Chattopadhyay, Head, High Energy Physics, SINP, India. We acknowledge the support from the research grants from SINP-DAE 12 Five year plan Trace, Ultratrace Analysis and Isotope Production (TULIP), Government of India.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Susanta Lahiri.

Additional information

Communicated by Navin Alahari

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Choudhury, D., Lahiri, S., Naskar, N. et al. Quantification of radioisotopes produced in 1.4 GeV proton irradiated lead–bismuth eutectic targets. Eur. Phys. J. A 56, 204 (2020). https://doi.org/10.1140/epja/s10050-020-00191-z

Download citation

  • Received:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1140/epja/s10050-020-00191-z

Navigation