Spin-density-wave state in (TMTSF)2PF6: A 77Se NMR study at high magnetic fields

S. Valfells, P. Kuhns, A. Kleinhammes, J. S. Brooks, W. Moulton, S. Takasaki, J. Yamada, and H. Anzai
Phys. Rev. B 56, 2585 – Published 1 August 1997
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Abstract

We present a nuclear magnetic resonance study of the low-temperature spin-density-wave (SDW) ground state in the quasi-one-dimensional conductor (TMTSF)2PF6 [bis-(tetramethyl-tetraselenafulvalene)hexafluorophosphate]. Using magnetic fields up to 22 T, we have measured the 77Se spin-lattice (T11) and spin-spin relaxation rates (T21) above and below the SDW transition (TSDW12 K). Between TSDW and 4 K, we observe anomalously fast and Korringa-like T11; below 4 K, T11 decays rapidly. A reduction in T21 is also observed at 4 K, but the absorption linewidth does not change to within experimental error. We attribute this behavior to an incomplete SDW transition at TSDW, leaving residual carriers at the Fermi level, and a subsequent consummation of the transition at 4 K. Our data below 4 K are consistent with a simple model of the temperature dependence of T11 in a fully gapped and low-dimensional conductor.

  • Received 14 November 1996

DOI:https://doi.org/10.1103/PhysRevB.56.2585

©1997 American Physical Society

Authors & Affiliations

S. Valfells

  • Department of Physics, Boston University, Boston, Massachusetts 02215

P. Kuhns and A. Kleinhammes

  • National High Magnetic Field Laboratory, 1800 East Paul Dirac Drive, Tallahassee, Florida 32310

J. S. Brooks

  • Department of Physics, Boston University, Boston, Massachusetts 02215;
  • National High Magnetic Field Laboratory, 1800 East Paul Dirac Drive, Tallahassee, Florida 32310;
  • Department of Physics, Florida State University, Tallahassee, Florida 32306-4005

W. Moulton

  • National High Magnetic Field Laboratory, 1800 East Paul Dirac Drive, Tallahassee, Florida 32310
  • Department of Physics, Florida State University, Tallahassee, Florida 32306-4005

S. Takasaki, J. Yamada, and H. Anzai

  • Himeji Institute of Technology, 2167 Shosya, Himeji, Hyogo 671-22, Japan

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Vol. 56, Iss. 5 — 1 August 1997

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