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2020RO18      Phys.Rev. C 102, 044613 (2020)

A.K.H.Robertson, P.Kunz, C.Hoehr, P.Schaffer

Nuclide production cross sections from irradiation of thorium by 438 MeV protons and a comparison to fluka and geant4 simulations

NUCLEAR REACTIONS ²³²Th(p, X)⁸³Rb/⁸⁸Y/⁹⁵Nb/⁹⁵Zr/⁹⁹Mo/¹⁰³Ru/¹⁰⁵Rh/¹⁰⁶Ru/^110mAg/¹¹¹In/¹¹¹Ag/^114mIn/¹¹⁵Cd/^120mSb/¹²¹Te/^121mTe/¹²²Sb/¹²⁴Sb/¹²⁵Sb/¹²⁵Sn/¹²⁶Sb/¹²⁷Sb/¹³¹Ba/¹³²Te/¹³⁴Cs/¹³⁶Cs/¹³⁹Ce/¹⁴⁰Ba/¹⁴¹Ce/¹⁴⁴Ce/²⁰¹Tl/²⁰³Pb/²⁰⁵Bi/²⁰⁶Po/²⁰⁶Bi/²⁰⁷Bi/²²³Ra/²²⁴Ra/²²⁵Ac/²²⁵Ra/²²⁶Ac/²²⁷Ac/²²⁷Th/²²⁸Ra/²²⁸Th/²³⁰Pa/²³³Pa, E=438 MeV from TRIUMF cyclotron; measured off-line Eγ, Iγ; deduced total radioactivity and production σ for 38 out of 47 radioactive isotopes measured and produced in spallation and high-energy fission reactions. Comparison to simulated cross sections calculated using three Monte Carlo computer codes: FLUKA, GEANT4 with Liege intranuclear cascade model, GEANT4 with the binary cascade model, and ABLA evaporation code. Relevance to the production of ²²⁵Ac isotope, a radionuclide of interest in nuclear medicine for the treatment of cancer.

doi: 10.1103/PhysRevC.102.044613
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