212FR    216AC A DECAY (440 US)        2004Ku24                  20NDS    202009
212FR  H TYP=FUL$AUT=K. Auranen and E.A. McCutchan$CIT=NDS 168, 117 (2020)$
212FR2 H CUT=1-Aug-2020$
212FR c  2004Ku24: the nuclei of interest were produced in the
212FR2c  fusion-evaporation reaction {+209}Bi({+12}C,5n). The 240-|mg/cm{+2}
212FR3c  thick targets had a 40-|mg/cm{+2} thick carbon backing. The {+12}C
212FR4c  beam was provided by the UNILAC accelerator at the energy of 7.1
212FR5c  MeV/nucleon and at the intensity of |?200 pnA. Residues were selected
212FR6c  with the velocity filter SHIP, and those were implanted into 16-strip
212FR7c  PIPS Si detector with a HPGe detector mounted immediately behind.
212FR8c  E|g, E|a, I|g, I|a, |g|a coincidences were measured.
212FR c  Others: 1968Va18, 1970To18, 2000He17, 2005Li17, 2018Hu13
212FR cA E$From 2004Ku24
212FR cA IA$Deduced indirectly by 2004Ku24 from |a|g coincidences by
212FR2cA normalizing the number of |g-ray counts to those of |a- and |g-lines
212FR3cA observed for the 853 and 938 levels (which yielded identical values),
212FR4cA unless stated otherwise. Uncertainties for intensities obtained by
212FR5cA this method are statistical only. Plausible effect due to summing of
212FR6cA |a-particle and conversion electrons were not taken into account,
212FR7cA meaning the quoted I{-|a} values are lower or upper limits as
212FR8cA indicated.
212FR cL E$From a least-square fit to the E|g data by the evaluator
212FR cL J,T$From the Adopted Levels.
212FR cA HF$r{-0}({+212}Fr)=1.5043 {I22}, average of r{-0}({+212}Ra)=1.4695
212FR2cA {I14}, r{-0}({+214}Ra)=1.5487 {I30}, r{-0}({+210}Rn)=1.4557 {I12}, and
212FR3cA r{-0}({+212}Rn)=1.5433 {I36} (2020Si16).
212FR c  $The {+212}Fr level scheme and {+216}Ac |a-decay data adopted here
212FR2c  follows that presented in 2004Ku24.
212FR c  In the previous A=212 evaluation (2005Br03) four excited states were
212FR2c  adopted for {+212}Fr based on |a feeding from a low-lying (47 keV
212FR3c  {I11}), high-spin (9{+-}) isomeric state of {+216m}Ac with a
212FR4c  half-life nearly identical to that of the {+216}Ac ground state, see,
212FR5c  i.e. 1968Va18, 1970To18, 2000He17. Later, in 2004Ku24, based on |a|g
212FR6c  coincidence measurement it was obseved that all Q{-|a}+E{-|g} sums
212FR7c  are equal to the Q{-|a} of  the g.s. to g.s. |a decay, and that a
212FR8c  change in beam energy did not have an impact on the relative
212FR9c  population of the {+216}Ac ground state and assumed isomer.
212FRac  Furthermore, in 2004Ku24 it was pointed out that the obtained
212FRbc  |a-decay hindrance factors do not support high-spin origin, but
212FRcc  instead all observed |a decays can be explained by the (1{+-}) ground
212FRdc  state of {+216}Ac. Consequently, the assignment of a high-spin isomer
212FRec  in {+216}Ac is considered erroneous, and the respective {+212}Fr
212FRfc  levels, as well as the corresponding {+216m}Ac |a-decay data set were
212FRgc  removed in the present evaluation.
212FR cG E,RI$From 2004Ku24. Intensities are normalized to 100 for the most
212FR2cG intense |g-ray from each level.
212FR cG M$From the Adopted Levels. For cases where the multipolarity derives
212FR2cG from this dataset, supporting evidence is given in the comments.
212FR D  CC$FROM BrIcc v2.3b (16-Dec-2014) 2008Ki07, "Frozen Orbitals" appr.
216AC  P 0.0          (1-)              440 US    16             9235     6
216AC cP T$from 2000He17. Other: 390 |ms {I60} (2005Li17)
216AC cP J$analogy with {+212}At and {+214}Fr
212FR  N                        1
212FR PN                                                                     7
212FR  G 406.2     1
212FR  G 617.3     3
212FR  G 765.3     2
212FR  G 1081.3    3
212FR  L 0.0          5+                20.0 M    6
212FR  A 9105      7 47.5    5 235     14
212FR cA IA$deduced from the singles |a-spectrum by assuming the tail in the
212FR2cA 9029 |a transition towards higher energy is due to summing of 9029
212FR3cA keV |a-particles and conversion electrons from the 82 keV transition.
212FR4cA Other: 75 {I57} (2018Hu13).
212FR cA E$Others: 9052 keV {I10} (2000He17), 9070 {I50} (2005Li17),
212FR2cA 9070 keV {I8} (1970To18), 9069 {I6} (2018Hu13)
212FR  L 82.48     6  (4+)
212FR  G 82.6      1  100                                                    C
212FR  A 9029      7 48.8    10145     9
212FR cA IA$deduced from the singles |a-spectrum by assuming the tail in the
212FR2cA 9029 |a transition towards higher energy is due to summing of 9029
212FR3cA keV |a-particles and conversion electrons from the 82 keV transition.
212FR4cA Other: 25 {I28} (2018Hu13)
212FR cA E$others: 8990 keV {I20} (1970To18), 8976 {I10} (2018Hu13)
212FR  L 500.72    7
212FR  G 418.3     1  100    6                                               C
212FR  G 500.7     1  53     4
212FR  A 8616      6 0.23    5 2.69E3  61
212FR cA IA$from the singles |a-spectrum.
212FR  L 536.34    8
212FR  G 453.9     1  9      1                                               C
212FR  G 536.3     1  100    6
212FR  A 8581      6 0.51    GT1.03E3  LT
212FR cA IA$|DI|a=0.06
212FR  L 542.00    10 7+
212FR  G 542.0     1  100       E2                      0.0305
212FR  A 8576      6 0.46    GT1108    LT
212FR cA IA$|DI|a=0.05
212FR  L 574.89    11
212FR  G 492.4     1  100    4                                               C ?
212FR  G 575.0     4  1.3    4                                                 ?
212FR  A 8536      150.12    GT3474    LT
212FR cA IA$|DI|a=0.02
212FR  L 606.23    8
212FR  G 105.8     2  11     3                                               C
212FR  G 523.7     1  100    7                                               C
212FR  G 606.2     1  60     7
212FR  A 8514      6 0.11    GT3125    LT
212FR cA IA$|DI|a=0.02
212FR  L 610.60    20
212FR  G 610.6     2  100
212FR  A 8509      7 0.017   GT19684   LT
212FR cA IA$|DI|a=0.001
212FR  L 777.29    10
212FR  G 276.6     2  1.3    6
212FR  G 694.8     1  100    5                                               C
212FR  G 777.3     2  14     2
212FR  A 8346      7 0.1     LT1050    GT
212FR  L 853.73    8  (4+,5+,6+)
212FR  G 352.9     2  1.2    5                                               C
212FR  G 771.3     1  77     4                                               C
212FR  G 853.7     1  100    4  (M1)                    0.0397
212FRX G EKC=0.06 6
212FRS G KC=0.0322 5$LC=0.00569 8$MC=0.001348 19$NC=0.000353 5$OC=7.90E-5 11$
212FRS G PC=1.269E-5 18$QC=7.13E-7 10
212FR cG EKC$deduced by gating on |a-particles with energies between 8230 and
212FR2cG 8320.
212FR  A 8270      5 1.40    7 49      4
212FR cA IA$from the singles |a-spectrum.
212FR  L 938.21    10 (4+,5+,6+)
212FR  G 855.8     7  5      LE                                              C
212FR  G 938.2     1  100    2  (M1)                    0.0310
212FRX G EKC=0.027 17
212FRS G KC=0.0252 4$LC=0.00443 7$MC=0.001051 15$NC=0.000275 4$OC=6.16E-5 9$
212FRS G PC=9.90E-6 14$QC=5.57E-7 8
212FR cG EKC$deduced from ratio between L{-|a1} x-rays and 938 |g-rays gated
212FR2cG by the 8187 |a-transition.
212FR  A 8187      5 0.74    2 53      4
212FR cA IA$from the singles |a-spectrum.
212FR  L 1008.7    4
212FR  G 1008.7    4  100
212FR  A 8114      9 0.0020  GT13023   LT
212FR cA IA$|DI|a=0.0003
212FR  L 1129.9    5
212FR  G 1047.5    9  85     50
212FR  G 1129.9    5  100    40
212FR  A 8001      150.0024  GT4792    LT
212FR cA IA$|DI|a=0.0016
212FR  L 1209.5    5
212FR  G 1209.5    5  100
212FR  A 7924      150.0013  GT5116    LT
212FR cA IA$|DI|a=0.0002
212FR  L 1239.9    4
212FR  G 1239.9    4  100
212FR  A 7892      100.021   2 242     27
212FR cA IA$from the singles |a-spectrum.
212FR  L 1287.1    8
212FR  G 1287.1    8  100
212FR  A 7846      150.016   3 229     45
212FR cA IA$from the singles |a-spectrum.
212FR  L 1356.0    20
212FR  G 1356      2  100
212FR  A 7776      150.0010  GT2372    LT
212FR cA IA$|DI|a=0.0004
212FR  L 1375.35   23
212FR  G 436.8     6  17     6
212FR  G 1293.1    4  45     17
212FR  G 1375.3    3  100    20
212FR  A 7758      6 0.011   3 177     50
212FR cA IA$from the singles |a-spectrum.