Microscopic description of fission in uranium isotopes with the Gogny energy density functional

R. Rodríguez-Guzmán and L. M. Robledo
Phys. Rev. C 89, 054310 – Published 8 May 2014

Abstract

The most recent parametrizations D1S, D1N, and D1M of the Gogny energy density functional are used to describe fission in the isotopes 232280U. Fission paths, collective masses, and zero-point quantum corrections, obtained within the constrained Hartree-Fock-Bogoliubov approximation, are used to compute the systematics of the spontaneous fission half-lives tSF, the masses and charges of the fission fragments, and their intrinsic shapes. The Gogny-D1M parametrization has been benchmarked against available experimental data on inner and second barrier heights, excitation energies of the fission isomers, and half-lives in a selected set of Pu, Cm, Cf, Fm, No, Rf, Sg, Hs, and Fl nuclei. It is concluded that D1M represents a reasonable starting point to describe fission in heavy and superheavy nuclei. Special attention is also paid to understand the uncertainties in the predicted tSF values arising from the different building blocks entering the standard semiclassical Wentzel-Kramers-Brillouin formula. Although the uncertainties are large, the trend with mass or neutron numbers are well reproduced and therefore the theory still has predictive power. In this respect, it is also shown that modifications of a few percent in the pairing strength can have a significant impact on the collective masses leading to uncertainties in the tSF values of several orders of magnitude.

  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
9 More
  • Received 27 December 2013
  • Revised 28 March 2014

DOI:https://doi.org/10.1103/PhysRevC.89.054310

©2014 American Physical Society

Authors & Affiliations

R. Rodríguez-Guzmán*

  • Department of Physics and Astronomy, Rice University, Houston, Texas 77005, USA and Department of Chemistry, Rice University, Houston, Texas 77005, USA

L. M. Robledo

  • Departamento de Física Teórica, Universidad Autónoma de Madrid, 28049 Madrid, Spain

  • *raynerrobertorodriguez@gmail.com
  • luis.robledo@uam.es

Article Text (Subscription Required)

Click to Expand

References (Subscription Required)

Click to Expand
Issue

Vol. 89, Iss. 5 — May 2014

Reuse & Permissions
Access Options
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×
×

Images

×

Sign up to receive regular email alerts from Physical Review C

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×