Mass distribution in the 50-, 60-, and 70-MeV bremsstrahlung-induced fission of 232Th

H. Naik, T. N. Nathaniel, A. Goswami, G. N. Kim, M. W. Lee, S. V. Suryanarayana, S. Ganesan, E. A. Kim, M.-H. Cho, and K. L. Ramakumar
Phys. Rev. C 85, 024623 – Published 27 February 2012; Erratum Phys. Rev. C 85, 039905 (2012)

Abstract

The postneutron yields of various fission products in the mass regions of 77–153 have been determined in the 50-, 60-, and 70-MeV bremsstrahlung-induced fission of 232Th by using a recoil catcher and an off-line γ-ray spectrometric technique in the electron linac at the Pohang Accelerator Laboratory, Korea. The mass-yield distributions were obtained from the fission-product yield data using charge-distribution corrections. The fission yields of the present paper and the existing data from the 232Th(γ,f) reaction at various energies are compared with those from the 232Th(n,f), the 238U(n,f), and the 238U(γ,f) reactions. We observe that the yields of fission products for A = 133-134, A = 138-139, A = 143-144, and their complementary products in the above fissioning systems are higher than those of other fission products, which is explained based on the nuclear-structure effect. However, we observed that the yields of fission products for A = 133-134 were lower than those for A = 143-144 in the 232Th(γ,f) reaction compared to those of the 232Th(n,f), 238U(n,f), and 238U(γ,f) reactions. The yields of fission products for A = 133-134 increase, but those for A = 143-144 decrease with an increase in the excitation energy in the 232Th(γ,f) and 232Th(n,f) reactions; however, those trends are reversed in the 238U(γ,f) and 238U(n,f) reactions. The increasing or decreasing trends for the yields of fission products for A = 133-134 and A = 143-144 with the excitation energy in the 232Th(γ,f), 232Th(n,f), 238U(n,f), and 238U(γ,f) reactions are explained from the shell effect of the complementary products based on the static scission-point model and the standard I and II channels of bimodal fission. The peak-to-valley (P/V) ratio for the above fissioning systems also was obtained from the mass-yield distribution. The P/V ratio for the 232Th(γ,f) and 238U(γ,f) reactions at different energies from the present data and the existing literature data are interpreted to examine the role of excitation energy.

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  • Received 27 December 2011

DOI:https://doi.org/10.1103/PhysRevC.85.024623

©2012 American Physical Society

Erratum

Erratum: Mass distribution in the 50-, 60-, and 70-MeV bremsstrahlung-induced fission of 232Th [Phys. Rev. C 85, 024623 (2012)]

H. Naik, T. N. Nathaniel, A. Goswami, G. N. Kim, M. W. Lee, S. V. Suryanarayana, S. Ganesan, E. A. Kim, M.-H. Cho, and K. L. Ramakumar
Phys. Rev. C 85, 039905 (2012)

Authors & Affiliations

H. Naik, T. N. Nathaniel, and A. Goswami

  • Radiochemistry Division, Bhabha Atomic Research Centre, Mumbai 400085, India

G. N. Kim* and M. W. Lee

  • Department of Physics, Kyungpook National University, Daegu 702-701, Republic of Korea

S. V. Suryanarayana

  • Nuclear Physics Division, Bhabha Atomic Research Centre, Mumbai 400085, India

S. Ganesan

  • Reactor Physics Design Division, Bhabha Atomic Research Centre, Mumbai 400085, India

E. A. Kim and M.-H. Cho

  • Division of Advanced Nuclear Engineering, Pohang University of Science and Technology, Pohang 790-784, Republic of Korea

K. L. Ramakumar

  • Radiochemistry and Isotope Group, Bhabha Atomic Research Centre, Mumbai 400085, India

  • *gnkim@knu.ac.kr

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Vol. 85, Iss. 2 — February 2012

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