Skip to main content
Log in

Startup of superheavy element chemistry at RIKEN

  • Chemical Properties of the Heaviest Elements
  • Published:
The European Physical Journal D Aims and scope Submit manuscript

Abstract.

A review is given on the startup of the superheavy element (SHE) chemistry at RIKEN. A gas-jet transport system for the SHE chemistry has been coupled to the gas-filled recoil ion separator GARIS at the RIKEN Linear Accelerator. The performance of the system was appraised using 206Fr and 245Fm produced in the 169Tm (40Ar, 3n) 206Fr and 208Pb (40Ar, 3n) 245Fm reactions, respectively. The α particles of 206Fr and 245Fm separated with GARIS and transported by the gas-jet were identified with a rotating wheel system for α spectrometry under desired low background condition. The high gas-jet efficiencies over 80% were independent of the beam intensities up to 2 particle μA. A gas-jet coupled target system for the production of SHEs was also installed on the beam line of the RIKEN K70 AVF cyclotron. The gas-jet transport of 255No and 261Rf produced in the 238U (22Ne, 5n) 255No and 248Cm (18O, 5n) 261Rf reactions, respectively, was conducted for the future chemical studies of 265Sg via the 248Cm (22Ne, 5n) 265Sg reaction.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  • The Chemistry of Superheavy Elements, edited by M. Schädel (Kluwer Academic Publishers, Dordrecht, 2003)

  • M. Schädel, Angew. Chem. Int. Ed. 45, 368 (2006)

    Article  Google Scholar 

  • P. Pyykkö, Chem. Rev. 88, 563 (1988)

    Article  Google Scholar 

  • V.G. Pershina, Chem. Rev. 96, 1977 (1996)

    Article  Google Scholar 

  • Y. Nagame, K. Tsukada, M. Asai, A. Toyoshima, K. Akiyama, Y. Ishii, T. Kaneko-Sato, M. Hirata, I. Nishinaka, S. Ichikawa, H. Haba, S. Enomoto, K. Matsuo, D. Saika, Y. Kitamoto, H. Hasegawa, Y. Tani, W. Sato, A. Shinohara, M. Ito, J. Saito, S. Goto, H. Kudo, H. Kikunaga, N. Kinoshita, A. Yokoyama, K. Sueki, Y. Oura, H. Nakahara, M. Sakama, M. Schädel, W. Brüchle, J.V. Kratz, Radiochim. Acta 93, 519 (2005)

    Article  Google Scholar 

  • 6th Workshop on Recoil Separator for SHE Chemistry, September 29, 2006, Garching, Germany, http://www-w2k.gsi.de/tasca06/

  • J.P. Omtvedt, J. Alstad, H. Breivik, J.E. Dyve, K. Eberhardt, C.M. Folden III, T. Ginter, K.E. Gregorich, E.A. Hult, M. Johansson, U.W. Kirbach, D.M. Lee, M. Mendel, A. Nähler, V. Ninov, L.A. Omtvedt, J.B. Partin, G. Skarnemark, L. Stavsetra, R. Sudowe, N. Wiehl, B. Wierczinski, P.A. Wilk, P.M. Zielinski, J.V. Kratz, N. Trautmann, H. Nitsche, D.C. Hoffman, J. Nucl. Radiochem. Sci. 3, 121 (2002)

    Google Scholar 

  • L. Stavsetra, K.E. Gregorich, J. Alstad, H. Breivik, K. Eberhardt, C.M. Folden III, T.N. Ginter, M. Johansson, U.W. Kirbach, D.M. Lee, M. Mendel, L.A. Omtvedt, J.B. Patin, G. Skarnemark, R. Sudowe, P.A. Wilk, P.M. Zielinski, H. Nitsche, D.C. Hoffman, J.P. Omtvedt, Nucl. Instr. Meth. A 543, 509 (2005)

    Article  ADS  Google Scholar 

  • Ch.E. Düllmann, G.K. Pang, C.M. Folden III, K.E. Gregorich, D.C. Hoffman, H. Nitsche, R. Sudowe, P.M. Zielinski, in Advances in Nuclear and Radiochemistry, General and Interdisciplinary, edited by S.M. Qaim, H.H. Coenen (Forschungszentrum Jülich GmbH, Jülich, 2004), Vol. 3, p. 147

  • Ch.E. Düllmann, C.M. Folden III, K.E. Gregorich, D.C. Hoffman, D. Leitner, G.K. Pang, R. Sudowe, P.M. Zielinski, H. Nitsche, Nucl. Instr. Meth. A 551, 528 (2005)

    Article  ADS  Google Scholar 

  • R. Sudowe, M.G. Galvert, Ch.E. Düllmann, L.M. Farina, C.M. Folden III, K.E. Gregorich, S.E.H. Gallaher, D.C. Hoffman, S.L. Nelson, D.C. Phillips, J.M. Schwantes, R.E. Wilson, P.M. Zielinski, H. Nitsche, Radiochim. Acta 94, 123 (2006)

    Article  Google Scholar 

  • U.W. Kirbach, C.M. Folden III, T.N. Ginter, K.E. Gregorich, D.M. Lee, V. Ninov, J.P. Omtvedt, J.B. Patin, N.K. Seward, D.A. Strellis, R. Sudowe, A. Türler, P.A. Wilk, P.M. Zielinski, D.C. Hoffman, H. Nitsche, Nucl. Instr. Meth. A 484, 587 (2002)

    Article  ADS  Google Scholar 

  • K. Morita, K. Morimoto, D. Kaji, H. Haba, E. Ideguchi, J.C. Peter, R. Kanungo, K. Katori, H. Koura, H. Kudo, T. Ohnishi, A. Ozawa, T. Suda, K. Sueki, I. Tanihata, H. Xu, A.V. Yeremin, A. Yoneda, A. Yoshida, Y.-L. Zhao, T. Zheng, S. Goto, F. Tokanai, J. Phys. Soc. Jpn 73, 1738 (2004)

    Article  ADS  Google Scholar 

  • K. Morita, K. Morimoto, D. Kaji, H. Haba, E. Ideguchi, R. Kanungo, K. Katori, H. Koura, H. Kudo, T. Ohnishi, A. Ozawa, T. Suda, K. Sueki, I. Tanihata, H. Xu, A.V. Yeremin, A. Yoneda, A. Yoshida, Y.-L. Zhao, T. Zhen, Eur. Phys. J. A 21, 257 (2004)

    Article  ADS  Google Scholar 

  • K. Morita, K. Morimoto, D. Kaji, T. Akiyama, S. Goto, H. Haba, E. Ideguchi, H. Koura, H. Kudo, T. Ohnishi, A. Ozawa, T. Suda, K. Sueki, H. Xu, T. Yamaguchi, A. Yoneda, A. Yoshida, Y.-L. Zhao, RIKEN Accel. Prog. Rep. 38, 69 (2005)

    Google Scholar 

  • K. Morita, K. Morimoto, D. Kaji, T. Akiyama, S. Goto, H. Haba, E. Ideguchi, R. Kanungo, K. Katori, H. Koura, H. Kudo, T. Ohnishi, A. Ozawa, T. Suda, K. Sueki, H. Xu, T. Yamaguchi, A. Yoneda, A. Yoshida, Y.-L. Zhao, J. Phys. Soc. Jpn 73, 2593 (2004)

    Article  ADS  Google Scholar 

  • D. Vermeulen, H.-G. Clerc, C.-C. Sahm, K.-H. Schmidt, J.G. Keller, G. Münzenberg, W. Reisdorf, Z. Phys. A 318, 157 (1984)

    Article  Google Scholar 

  • J.M. Nitschke, R.E. Leber, M.J. Nurmia, A. Ghiorso, Nucl. Phys. A 313, 236 (1979)

    Article  ADS  Google Scholar 

  • Y. Nagame, M. Asai, H. Haba, S. Goto, K. Tsukada, I. Nishinaka, K. Nishio, S. Ichikawa, A. Toyoshima, K. Akiyama, H. Nakahara, M. Sakama, M. Schädel, J.V. Kratz, H.W. Gäggeler, A. Türler, J. Nucl. Radiochem. Sci. 3, 85 (2002)

    Google Scholar 

  • R.B. Firestone, V.S. Shirley, Table of Isotopes, 8th edn. (John Wiley and Sons, New York, 1996)

  • E.D. Donets, V.A. Shchegolev, V.A. Ermakov, Sov. J. Nucl. Phys. 2, 723 (1966)

    Google Scholar 

  • M. Asai, K. Tsukada, M. Sakama, S. Ichikawa, T. Ishii, Y. Nagame, I. Nishinaka, K. Akiyama, A. Osa, Y. Oura, K. Sueki, M. Shibata, Phys. Rev. Lett. 95, 102502 (2005)

    Article  ADS  Google Scholar 

  • D. Saika, Y. Kitamoto, K. Matsuo, Y. Tashiro, T. Takabe, T. Yoshimura, W. Sato, N. Takahashi, H. Haba, S. Enomoto, A. Shinohara, RIKEN Accel. Prog. Rep. 39, 111 (2006)

    Google Scholar 

  • A. Toyoshima, Y. Kasamatsu, A. Kitatsuji, K. Tsukada, H. Haba, A. Shinohara, Y. Nagame, J. Nucl. Radiochem. Sci. (to be published)

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to H. Haba.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Haba, H., Akiyama, T., Kaji, D. et al. Startup of superheavy element chemistry at RIKEN. Eur. Phys. J. D 45, 81–86 (2007). https://doi.org/10.1140/epjd/e2007-00135-4

Download citation

  • Received:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1140/epjd/e2007-00135-4

PACS.

Navigation