Elsevier

Nuclear Physics A

Volume 562, Issue 2, 20 September 1993, Pages 205-217
Nuclear Physics A

Measurements of spectroscopic quadrupole moments of neutron-deficient Au isotopes with quadrupole-interaction-resolved NMR-ON

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Abstract

We report on measurements of quadrupole-interaction-resolved nuclear magnetic resonance on oriented nuclei (QI-NMR-ON) of 32+ 193Au (T12 = 17.5 h)and 32+ 195Au(T12=183 d) hcp-Co. The results for the magnetic and electric hyperfine splittings are: 193Au: νM = 67.72(2) MHz;νQ = − 15.69(4) MHz;195Au; νM = 71.65(1) MHz; νQ = − 14.34(2) MHz. Taking into account hyperfine anomalies, the magnetic moments are deduced to be: μ(193Au) = 0.1396(6) μN; μ(195Au) = 0.1487(6) μN. With the known quadrupole moment of 193Au, Q = + 0.664(20), b, the electric field gradient of Au in hcp-Co is deduced to be eq = − 0.977(29) × 1017 V/cm2, with which Q(195Au) = + 0.607(18) b is obtained for the spectroscopic quadrupole moment of 195Au. In addition, the experimentally known quadrupole splitting frequencies of 186Au, 198Au and 199Au in hcp-Co can be reinterpreted, giving the results: Q(186Au) = + 3.14(16) b; Q(198Au) = + 0.640(19) b; Q(199Au) = + 0.510(16) b.

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