Levels in Pu237 populated by Am237 (electron capture) and Cm241(α) decays

I. Ahmad, F. T. Porter, M. S. Freedman, R. K. Sjoblom, J. Lerner, R. F. Barnes, J. Milsted, and P. R. Fields
Phys. Rev. C 12, 541 – Published 1 August 1975
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Abstract

The electron capture decay scheme of Am237 (73 min) has been investigated by measuring the γ-ray and conversion-electron spectra of mass-separated Am237 samples. The γ-ray spectra were measured with a Ge(Li) spectrometer and the conversion-electron spectra were measured with a cooled Si(Li) detector and a magnetic β-ray spectrometer. Thirty-five γ rays were identified and the multipolarities of most of the transitions were deduced. The half-life of Am237 was determined by following the decay of the 280.2 keV photopeak and was found to be 73.0 ± 1.0 min. The α-particle energy and α branching were measured to be 6.042 ± 0.005 MeV and [(2.5 ± 0.3) × 102]%, respectively. On the basis of the present investigation the following single-particle states have been identified in Pu237: 72[743], 0 ½+[631], 145.5; 52+[622], 280.2; 32+[631], 370.4; 52+[633], 407.8; 72+[624], 473.5; 52[752], 655.3; and 72+[613], 908.8 keV. The ground state of Am237 has been deduced to be the 52[523] Nilsson orbital. The logft values for electron capture transitions to the observed states were derived. The α-particle spectrum of a mass-separated Cm241 sample was measured with the Argonne double focusing magnetic spectrometer. Eleven α groups identified in this spectrum populate the members of the ground state, ½+[631], and 32+[631] bands. The α-decay hindrance factors are consistent with the Nilsson-state assignments deduced from Am237 electron capture decay.

RADIOACTIVITY Am237 [from Np237(α, 4n) and Np237(He3, 3n))]; measured T12, Eα, Eγ, Iγ, Ece, Ice, γγ- coin, α branching, Cm241 [from Pu239(α, 2n)]; measured Eα, Iα; deduced hindrance factors. Pu237 deduced levels logft, (EC) γ multipolarity, I, π, eight single-particle states. Mass-separated Am237 and Cm241. Toroidal β spectrometer at 0.15% FWHM.

  • Received 21 April 1975

DOI:https://doi.org/10.1103/PhysRevC.12.541

©1975 American Physical Society

Authors & Affiliations

I. Ahmad, F. T. Porter, M. S. Freedman, R. K. Sjoblom, J. Lerner, R. F. Barnes, J. Milsted, and P. R. Fields

  • Chemistry Division, Argonne National Laboratory, Argonne, Illinois 60439

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Vol. 12, Iss. 2 — August 1975

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